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Arginine methylation of human DNA topoisomerase I by PRMT5 facilitates DNA relaxation - PubMed

3 hours ago
  • #Arginine Methylation
  • #PRMT5
  • #DNA Topoisomerase I
  • PRMT5 symmetrically dimethylates human DNA topoisomerase I (Top1) at arginine residues R708 and R749.
  • This methylation enhances Top1's DNA relaxation activity by improving strand rotation without affecting DNA binding.
  • Methylation-deficient Top1 mutants show impaired mobility, accumulate more Top1-DNA covalent complexes under camptothecin (CPT), and delay Top1cc resolution.
  • Loss of Top1 methylation, via mutation, PRMT5 knockout, or inhibitors, amplifies CPT-induced DNA damage.
  • Combining PRMT5 inhibitors with Top1 poisons like irinotecan increases cytotoxicity in cancer cells and suppresses tumor growth and metastasis in a mouse model.