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Glucose oxidase-mineralized scaffolds with multiple bioactivities for accelerated diabetic bone regeneration - PubMed

6 hours ago
  • #Biomineralization
  • #Bone Regeneration
  • #Diabetes
  • Engineered a biomimetic 3D-printed scaffold for diabetic bone regeneration.
  • Integrated glucose oxidase-mineralized amorphous calcium phosphate (GOx@ACP) nanoparticles into a gelatin methacryloyl (GelMA) hydrogel.
  • Biomineralization enhances enzymatic stability and enables glucose-responsive degradation.
  • Dual therapeutic actions: consumes glucose to alleviate hyperglycemia and generates trace H₂O₂ to promote angiogenesis.
  • Releases osteogenic ions (Ca²⁺/PO₄³⁻) upon ACP degradation.
  • Sustained degradation profile ensures matched release kinetics of ions and enzymes.
  • In vitro, enhances bone marrow stromal cell proliferation, osteogenic differentiation, and endothelial tubulogenesis.
  • In diabetic rat cranial defects, significantly accelerated bone regeneration with bone volume (BV/TV) reaching ~52% by the 12th week.